Bull. Chem. Soc. Jpn., 99
Bull. Chem. Soc. Jpn, 72, 207 (1999).

Ab Initio Molecular Orbital Study of Reaction of Pentafluoroethyl Radical with Hydroxyl and Hydrogen Radicals

Haruhiko Fukaya,* Taizo Ono, and Takashi Abe

Chemistry Department, National Industrial Research Institute of Nagoya Hirate-cho, Kita-ku, Nagoya 462-8510, Japan


Ab initio molecular orbital theory calculations have been carried out on the reactions of the pentafluoroethyl radical with the hydroxyl and the hydrogen radicals to estimate its fire suppression efficiency. It was found that pentafluoroethyl radical was more effective than trifluoromethyl radical: i.e. the former was easier to regenerate and more difficult to decompose than the latter. The differences between the zero-point energies calculated by the HF and the MP2 method were also described.
Last Modified: 2001/5/30
h.fukaya@aist.go.jp